Spin Susceptibility of Helical Carbon-Based Nanostructures with Almost Filled Band and Spin-Orbit Coupling
Journal of Superconductivity and Novel Magnetism(2024)
摘要
Some theoretical studies using perturbation and tight-binding methods have tried to shed light on the magnetic behaviors of carbon-based nanostructures in the limit of wave vector 𝐪=0 . In a recent work, we studied a half-filled model of helical carbon chains to gain new insights for 𝐪 0 . Although in carbon the energy bands are usually derived from partially filled atomic p-shells, here we explore the hole contribution to these magnetic responses. We calculate the longitudinal spin susceptibility of an almost-filled tight-binding model of a helical chain for 𝐪 0 . We find that when the Fermi level lies at the band edges, the system shows for positive chirality a divergent paramagnetic susceptibility. This result is in agreement with that previously reported for the macroscopic limit 𝐪=0 .
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关键词
Chiral nanostructures,Spin-orbit coupling,Magnatic susceptibility,Tight-binding approximation,Helical coordinates
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