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Where Dust Comes From: Global Assessment of Dust Source Attributions with AeroCom Models

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES(2024)

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摘要
The source of dust in the global atmosphere is an important factor to better understand the role of dust aerosols in the climate system. However, it is a difficult task to attribute the airborne dust over the remote land and ocean regions to their origins since dust from various sources are mixed during long-range transport. Recently, a multi-model experiment, namely the AeroCom-III Dust Source Attribution (DUSA), has been conducted to estimate the relative contribution of dust in various locations from different sources with tagged simulations from seven participating global models. The BASE run and a series of runs with nine tagged regions were made to estimate the contribution of dust emitted in East- and West-Africa, Middle East, Central- and East-Asia, North America, the Southern Hemisphere, and the prominent dust hot spots of the Bod & eacute;l & eacute; and Taklimakan Deserts. The models generally agree in large scale mean dust distributions, however models show large diversity in dust source attribution. The inter-model differences are significant with the global model dust diversity in 30%-50%, but the differences in regional and seasonal scales are even larger. The multi-model analysis estimates that North Africa contributes 60% of global atmospheric dust loading, followed by Middle East and Central Asia sources (24%). Southern hemispheric sources account for 10% of global dust loading, however it contributes more than 70% of dust over the Southern Hemisphere. The study provides quantitative estimates of the impact of dust emitted from different source regions on the globe and various receptor regions including remote land, ocean, and the polar regions synthesized from the seven models. As the most abundant aerosol type in the Earth's atmosphere, mineral dust plays an important role in global climate by interacting with incoming and outgoing radiation, providing liquid and ice cloud nuclei, and affecting atmospheric stability. The global dust sources are relatively well characterized by the remote sensing and modeling studies as the majority of dust is emitted from the so-called dust belt which expands from North Africa to East Asia. However, it is challenging to attribute dust sources over the remote land and ocean regions, since dust is mixed during long-range transport, where it experiences complex atmospheric processes, including horizontal and vertical-advection, wet deposition, and dry deposition. Using the multi-model simulations in the Aerocom/Dust Source Attribution experiment, the present study (a) examines the model diversity in dust source attribution and (b) estimates the contribution of dust sources to various receptor regions, including remote land/ocean and the polar regions in different altitudes, from the multi-model statistics. Beyond dust sources, many remote land, ocean, and polar regions are affected by a mixture of dust from various sources around the globe. Contributions of various dust sources are quantitatively estimated in a multi-model experiment Contributions of various sources have different horizontal and vertical distributions and seasonality Dust near source regions are dominated by dust emitted in the upwind source regions; however many remote land, ocean, and polar regions are affected by a mixture of dust from various sources around the globe
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关键词
mineral dust,AeroCom,source attribution
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