Electrostatically fabricated heterostructure of interfacial-polarization-enhanced Fe3O4/C/MXene for ultra-wideband electromagnetic wave absorption
JOURNAL OF COLLOID AND INTERFACE SCIENCE(2024)
摘要
Electromagnetic (EM) pollution can disrupt the functioning of advanced electronic devices, hence it's necessary to design EM wave absorbers with high-level absorption capabilities. The Ti3C2Tx (MXene) is classified as a potential EM absorbing material; nevertheless, the lack of magnetic loss mechanism leads to its inadequate EM absorbing performance. On this basis, a novel composite design with promising EM absorption properties is hypothesized to be the integration of few-layer MXene and heterogeneous magnetic MOF derivatives (Fe3O4/C) with complementary advantages. Herein, we synthesized two-dimensional (2D) interfacial-polarizationenhanced MXene hybrid (Fe3O4/C/MXene) by electrostatic assembly. It is notable that the interfacial polarization is realized by adding a small amount of magnetic Fe3O4/C. Furthermore, the Fe3O4/C/ MXene demonstrates an astonishing effective absorption bandwidth (EAB) of 10.7 GHz and an excellent EM wave absorption performance (RLmin) of -66.9 dB. Moreover, the radar cross section (RCS) of Fe3O4/C/MXene is lower than -15.1 dB m2 from -90 degrees to 90 degrees with a minimum RCS value of -52.6 dB m2 at 32 degrees. In addition, the significant attenuation of the EM wave is due to the synergistic effect of improved impedance matching, dielectric loss, and magnetic loss. Thus, the magnetized Fe3O4/C/MXene hybrid is expected to emerge as a strong contender for high-performance EM wave absorbers.
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关键词
MXene,MOF derivative,Interfacial polarization,Ultra-wideband absorber,Radar cross section
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