Fission cross-section measurements for the 238U(n,f)97m+gNb, 238U(n, f)133gTe and 238U(n,f)130gSb reactions induced by D-T neutrons

Yafei Han, Yujie Qiao, Zhonglin Li, Xueyan Han,Qiang Wang,Kaihong Fang,Shuo Zhang

APPLIED RADIATION AND ISOTOPES(2024)

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摘要
In this study, we conducted measurements of the independent fission cross-sections of 238U(n, f)97m+gNb, 238U(n, f)133gTe reactions and the cumulative cross section of 238U(n, f)130gSb reactions induced by neutron at energies around 14 MeV, i.e., 14.1 +/- 0.3, 14.5 +/- 0.3 and 14.7 +/- 0.3 MeV. The measurement results were obtained by the neutron activation method in combination with off-line gamma-ray spectrometry techniques. The neutron flux was monitored on line by the accompanying alpha-particle from T(d, n)4He reaction, and the neutron energies were determined by the cross-section ratio of 90Zr(n, 2n)8+gZr to 93Nb(n, 2n)92mNb reactions. The independent fission cross-sections of the fission reactions were obtained by subtracting the influence of precursor nuclei or excited states. The obtained results are as follows: for 238U(n, f)97m+gNb, the independent cross sections are 1.0 +/- 0.89, 0.98 +/- 0.85 and 0.78 +/- 0.70 mb at the specified neutron energy points. For 238U(n, f)133gTe, the independent fission cross-sections are 26.8 +/- 2.8, 27.7 +/- 2.9 and 20.5 +/- 2.3 mb, respectively, at the same neutron energy points. As for 238U(n, f)130gSb, the obtained cumulative fission cross-sections are 5.35 +/- 0.58, 5.05 +/- 0.53 and 4.03 +/- 0.44 mb, respectively, at the specified neutron energy points.
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关键词
Cross section measurement,238U(n f) reaction,Neutron energies of 14.1,14.5 and 14.7 MeV,Fission products97m+gNb,133gTe,130gSb
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