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Enhancing Plasma-Catalytic Toluene Oxidation: Unraveling the Role of Lewis-acid Sites on Δ-Mno2

Zheng Bo,Mengyu Cao,Huihui Zhang,Yaolin Wang,Jianhua Yan,Kefa Cen,Kostya (Ken) Ostrikov,Xin Tu

Chemical Engineering Journal（2024）

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Abstract
•Plasma-catalytic oxidation of toluene over δ-MnO2 was investigated.•δ-MnO2 with a layered structure was synthesized using a metal–organic framework.•Well-defined δ-MnO2 with accessible inter-lamellar Lewis-acid sites was designed.•The interlayer-exposed δ-MnO2 performed best in plasma-catalytic toluene oxidation.•Lewis-acid sites in δ-MnO2 are the active sites for toluene oxidation.
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Key words
Plasma catalysis,Volatile organic compounds,Toluene oxidation,δ-MnO2,Lewis-acid site,Oxygen vacancies
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