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Photofission and Photoneutron Cross Sections for 238U and 232Th

15TH INTERNATIONAL CONFERENCE ON NUCLEAR DATA FOR SCIENCE AND TECHNOLOGY, ND2022(2023)

Horia Hulubei Natl Inst Phys & Nucl Engn IFIN HH | Chinese Acad Sci | Japan Atom Energy Agcy | Univ Politeh Bucharest | Lomonosov Moscow State Univ | Univ Bucharest | Kyoto Univ | Univ Oslo | Texas A&M Univ | Konan Univ | Univ Hyogo

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Abstract
A specific objective of the recent IAEA Coordinated Research Project on Photonuclear Data and Photon Strength Functions (Code F41032; Duration 2016-2019) has been to measure photonuclear cross-section data where needed, for unexplored nuclei and cases of discrepant existing data. A dedicated experimental campaign has been conducted at the laser Compton-scattering γ-ray source of the NewSUBARU synchrotron radiation facility of SPring8, Japan, where photoneutron reactions for 11 nuclei from 9 Be to 209 Bi have been investigated in the Giant Dipole Resonance energy region. The measurements followed the development of a flat-effi ciency moderated neutron detection array and the associated neutron-multiplicity sorting techniques. The IAEA CRP campaign has been followed at NewSUBARU by new measurements of photofission and photoneutron reactions on 238 U and 232 Th in the energy range of 5.87 MeV – 20.14 MeV. The neutron-multiplicity sorting of high-multiplicity fission neutron coincidence events has been performed using a dedicated energy dependent, multiple firing statistical treatment. The photoneutron (γ, x n) and photofission (γ, f x n) reactions have been discriminated by considering a Gaussian distribution of prompt-fission-neutrons (PFN) multiplicities predicted by the evaporation theory. We here provide preliminary experimental (γ, n), (γ, 2n) and (γ, F) cross sections, average energies of PFN and of photoneutrons emitted in (γ, n) and (γ, 2n) reactions, as well as the mean number of PFN per fission act. The new 238 U cross sections are compared with recent statistical-model calculations performed with the EMPIRE code on existing data.
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Neutron Imaging,Neutron Activation Analysis
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要点】:该研究通过在NewSUBARU同步辐射设施进行实验,测量了238U和232Th的 photofission 和 photoneutron 截面,为核数据和光子强度函数的IAEA协调研究项目提供了新的数据。

方法】:研究利用激光康普顿散射伽马射线源,发展了一种平面效率调制中子检测阵列和中子多重性排序技术,通过统计处理高多重性裂变中子符合事件,区分了 photoneutron 和 photofission 反应。

实验】:实验在NewSUBARU设施上进行,能量范围在5.87 MeV至20.14 MeV之间,使用了一种能量依赖的多重发射统计处理方法对高多重性裂变中子符合事件进行排序,得到了初步的实验数据,并将新的238U截面数据与使用EMPIRE代码进行的最新统计模型计算进行了比较。