Hysteresis-Free Solution-Processed 2-D MoS2 Flake-Thin-Film Transistors With Improved Operational Stability

An interface trap negatively affects the performance of a thin-film transistor (TFT). In the current study, we demonstrate hysteresis-free solution-processed MoS2 TFTs with a significantly reduced trap density of 3.7 x 10(10) cm(-2) using a poly(methylmethacrylate) (PMMA) dielectric in a top-gate top-contact (TGTC) device structure, which is much lower than that with a SiO2 back-gate dielectric layer (7.9 x 10(11) cm(-2)). The TFTs show a field-effect mobility of 7 cm(2)/V s for both forward and reverse scans, with an ON/ OFF current ratio of >106. In addition, after 3000 s of the bias-stress test, the drain current of the device degrades by only 7%.