Aconitine Synthesis Studies. A Modeling Construction of the Functionalized BCDE Tetracyclic Ring System

Tianyuan Guo,Fuli Peng, Xueqin Song,Jiang Lei, Fangzhou Yu, Hongping Chu, Keyang Yang,Liang Xu

Organic chemistry frontiers（2023）

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摘要

A highly functionalized BCDE model ring system of aconitine has been synthesized for the first time via a strategy involving oxidative dearomatization/IMDA, Wagner–Meerwein rearrangement, Michael addition and reductive cyclization.

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