Coherent Control of Single-Molecule Switching Reactions with Sub-Cycle Atomic Forces

Lukas Z. Kastner,Dominik Peller,Thomas Buchner,Carmen Roelcke,Florian Albrecht,Nikolaj Moll,Jascha Repp,Rupert Huber

2022 47th International Conference on Infrared, Millimeter and Terahertz Waves (IRMMW-THz)（2022）

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摘要

We introduce sub-cycle atomic-scale forces provided by near fields of a lightwave-driven scanning probe tip. Exerting these ultrafast forces to key atoms of a single-molecule switch allows us to coherently steer a select structural rotation that modulates the switching statistics by up to 39%.

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关键词

sub-cycle atomic forces,sub-cycle atomic-scale forces,lightwave-driven scanning probe tip,ultrafast forces,key atoms,single-molecule switch,switching statistics,coherent control,single-molecule switching reactions

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