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Effect of Ti Substitution on the Critical Behavior Around the Paramagnetic-Ferromagnetic Phase Transition of Pr0.75Bi0.05Sr0.1Ba0.1Mn1-xTixO3 (x=0, 0.02 and 0.04) Perovskite Compounds

Journal of alloys and compounds(2019)

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摘要
In this research work, our central focus is upon the investigation of the effect of the substitution of non magnetic Ti ions on the critical behavior of Pr0.75Bi0.05Sr0.1Ba0.1Mn1-xTixO3 (x = 0, 0.02 and 0.04) manganites. All our compounds underwent a second-order paramagnetic to ferromagnetic transition as temperature decreases. Several techniques such as modified Arrott plots, Kouvel-Fisher analysis and critical isotherm method were used in order to determine the values of the critical exponents beta, gamma and delta as well as the accurate Curie temperature T-C. The obtained values were found to be close to the 3D-Heisenberg model for the parent compound indicating a short-range inhomogeneous magnetic exchange coupling and to the mean-field model for doped samples describing long-range exchange interactions. We have also demonstrated that the universality class of the studied manganites was affected by Ti-doping. Besides, we highlighted that these parameters follow scaling equation with the magnetization data scaled into two different curves below and above (TC )confirming that the determined critical exponents and T-C are reasonably accurate. (C) 2019 Elsevier B.V. All rights reserved.
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关键词
Perovskite manganites,Titanium substitution,Critical field analysis,Scaling hypothesis
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