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Semi-classical Spin Dynamics of the Antiferromagnetic Heisenberg Model on the Kagome Lattice

Physical review B, Condensed matter and materials physics(2014)

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摘要
We investigate the dynamical properties of the classical antiferromagnetic Heisenberg model on the kagome lattice using a combination of Monte Carlo and molecular dynamics simulations. We find that frustration induces a distribution of time scales in the cooperative paramagnetic regime (i.e., far above the onset of coplanarity), as recently reported experimentally in deuterium jarosite. At lower temperature, when the coplanar correlations are well established, we show that the weather-vane loop fluctuations control the system relaxation: the time distribution observed at higher temperatures splits into two distinct time scales associated with fluctuations in the plane and out of the plane of coplanarity. The temperature and wave-vector dependencies of these two components are qualitatively consistent with loops diffusing in the entropically dominated free energy landscape. Numerical results are discussed and compared with the O(N) model and recent experiments for both classical and quantum realizations of the kagome magnets.
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