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Photooxidation by a long-lived photoexcited state of a triflic acid-bound Mn(IV)-oxo complex with the highest quantum efficiency

Rinny Kuilya,Young Hyun Hong,Namita Sharma,Yong-Min Lee,Wonwoo Nam,Shunichi Fukuzumi

Journal of Photochemistry and Photobiology A: Chemistry（2023）

Cited 1|Views7
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Abstract
This study reports a long-lived 2 E photoexcited state (τ = 21 µs) of metal-oxo complex composed of only earth-abundant elements, which oxidizes toluene by the two-photon four-electron oxidation process with ∼200% quantum efficiency that is the highest value ever reported.
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Key words
photoexcited state,long-lived,acid-bound
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