Giant reduced magnetic anisotropy in magneto-optical garnet

Magneto-optical garnet shows great potential in integrated optical isolators due to its highly efficient non-reciprocity. In this work, we prepared magneto-optical lithium-modified terbium bismuth iron garnet films using the liquid phase epitaxy method and systemically investigated the effect of lithium modification on magnetic properties. We found a trace amount of lithium modification induced in-plane magnetization and a minimum in-plane driving field around 2 Oe. Meanwhile, high remanence over 70% was obtained in tensile-strain samples. Most importantly, in comparison to unmodified samples, the calculation of anisotropy demonstrated the giant reduction of growth-induced anisotropy in the Li: TbBiIG up to 105erg/cm3. It reveals a new rule of ions’ preferred occupation in dodecahedral sublattices indirectly. This permits Furthermore, enhanced Faraday rotation in the near-infrared band was confirmed in the samples about 1 micrometer, up to 48% higher than unmodified samples. Our work shows Li:TbBiIGs enable a prime candidate material with substantial potential for integrated optical isolation applications.