Nitrous oxide activation by picoline-derived Ni-CNP hydrides

Jose Bermejo, Isabel Ortega-Lepe,Laura L. Santos,Nuria Rendon,Joaquin Lopez-Serrano,Eleuterio Alvarez,Andres Suarez

CHEMICAL COMMUNICATIONS（2024）

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摘要

Oxygen atom transfer (OAT) from N2O to the Ni-H bond of proton-responsive picoline-derived CNP nickel complexes has been investigated both experimentally and theoretically. These Ni-CNP complexes efficiently catalyse the reduction of N2O with pinacolborane (HBpin) under mild conditions. Picoline-derived Ni-CNP hydride complexes activate N2O upon base activation, and catalyse the reduction of N2O with pinacolborane.

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