A Universal Approach for Sustainable Urea Synthesis via Intermediate Assembly at the Electrode/Electrolyte Interface

Xiaojin Tu,Xiaorong Zhu,Shuowen Bo,Xiaoran Zhang,Ruping Miao,Guobin Wen,Chen Chen,Jing Li,Yangyang Zhou,Qinghua Liu,Dawei Chen,Huaiyu Shao,Dafeng Yan,Yafei Li,Jianfeng Jia,Shuangyin Wang

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION（2024）

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摘要

Electrocatalytic C-N coupling process is indeed a sustainable alternative for direct urea synthesis and co-upgrading of carbon dioxide and nitrate wastes. However, the main challenge lies in the unactivated C-N coupling process. Here, we proposed a strategy of intermediate assembly with alkali metal cations to activate C-N coupling at the electrode/electrolyte interface. Urea synthesis activity follows the trend of Li+更多

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关键词

C-N Coupling,Electrode/Electrolyte Interface,Intermediate Assembly,Urea Synthesis

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