Local distortion driven magnetic phase switching in pyrochlore Yb_2(Ti_1-xSn_x)_2O_7
arxiv(2024)
摘要
While it is commonly accepted that the disorder induced by magnetic ion
doping in quantum magnets usually generates a rugged free-energy landscape
resulting in slow or glassy spin dynamics, the disorder/distortion effects
associated with non-magnetic ion sites doping are still illusive. Here, using
AC susceptibility measurements, we show that the mixture of Sn/Ti on the
non-magnetic ion sites of pyrochlore Yb_2(Ti_1-xSn_x)_2O_7 induces an
antiferromagnetic ground state despite both parent compounds, Yb_2Ti_2O_7,
and Yb_2Sn_2O_7, order ferromagnetically. Local structure studies through
neutron total scattering reveals the local distortion in the non-magnetic ion
sites and its strong correlation with the magnetic phase switching. Our study,
for the first time, demonstrates the local distortion as induced by the
non-magnetic ion site mixture could be a new path to achieve magnetic phase
switching, which has been traditionally obtained by external stimuli such as
temperature, magnetic field, pressure, strain, light, etc.
更多查看译文
AI 理解论文
溯源树
样例
生成溯源树,研究论文发展脉络
Chat Paper
正在生成论文摘要