Nonlinear photocarrier dynamics in multilayer W S e 2 induced by intense terahertz pulses

Viela Guay,Nathan Johnson,Yue Zhang,Arend M. van der Zande, Spencer G. Thorp, M. J. Graham,Yun-Shik Lee

Journal of The Optical Society of America B-optical Physics(2023)

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摘要
Non-equilibrium photocarriers in multilayer WSe 2 injected by femtosecond laser pulses exhibit extraordinary nonlinear dynamics in the presence of intense THz fields. The THz absorption in optically excited WSe 2 rises rapidly in the low THz field regime and gradually ramps up at high intensities. The strong THz pulses drive the photocarriers into sidebands of higher mobility and release trapped charge carriers, which consequently enhance the transient conductivity of WSe 2 . The spectrally analyzed conductivity reveals distinctive features, indicating that the photocarriers undergo resonant interactions such as carrier-photon scattering.
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intense terahertz pulses
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