Breaking azeotropes by reactive adsorption: A case for sorption-enhanced dimethyl carbonate synthesis

Jasper van Kampen, Fabiënne Lucas,Martin van Sint Annaland

CHEMICAL ENGINEERING SCIENCE（2023）

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摘要

•SEDMC: direct synthesis of DMC from CO2 by in situ H2O adsorption.•SEDMC synthesis is an exemplary case for this reactive separation method.•Very high methanol conversions can be achieved compared to other direct synthesis routes.•The formation of two azeotropes can be avoided, simplifying downstream separation.

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关键词

Azeotropic product mixture,CO2 utilization,Dimethyl Carbonate,Reactive adsorption,Steam separation enhancement

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