Batch fabrication of MoS2 devices directly on growth substrates by step engineering
Nano Research(2023)
摘要
Monolayer molybdenum disulfide (MoS2) has emerged as one of the most promising channel materials for next-generation nanoelectronics and optoelectronics owing to its atomic thickness, dangling-bond-free flat surface, and high electrical quality. Currently, high-quality monolayer MoS2 wafers are primarily grown on sapphire substrates incompatible with conventional device fabrication, and thus transfer processes to a suitable substrate are typically required before the device can be processed. Here, we demonstrate the batch production of transfer-free MoS2 top-gate devices directly on sapphire growth substrates via step engineering. By introducing substrate steps on growth substrate sapphire, high-κ dielectric layers with superior quality and uniform can be directly deposited on the epitaxially grown monolayer MoS2. For the substrate with a maximum step density of 100 µm−1, the gate capacitance can reach ∼ 1.87 µF·cm−2, while the interface trap state density (Dit) can be as low as ∼ 7.6 × 1010 cm−2·eV−1. The direct deposition of high-quality dielectric layers on grown monolayer MoS2 enables the batch fabrication of top-gate devices devoid of transfer and thus excellent device yield of > 96
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关键词
substrate step engineering, atomic layer deposition, high-κ dielectric, molybdenum disulfide, top-gate field-effect transistor
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