Energetically preferred Li+ ion jump processes in crystalline solids: Site-specific hopping in β-Li3VF6 as revealed by high-resolution 6Li 2D EXSY NMR

Patrick Bottke,Katharina Hogrefe,Julia Kohl,Suliman Nakhal,Alexandra Wilkening,Paul Heitjans,Martin Lerch,H. Martin R． Wilkening

MATERIALS RESEARCH BULLETIN（2023）

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摘要

•2D EXSY NMR provides access to site-specific Li+ jump rates in β-Li3VF6.•Energetically preferred polyhedra connections are probed that lead to facile Li exchange.•Ranking in polyhedra configurations verifies current views from theory.

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关键词

NMR,Self-diffusion,Cathode materials,Exchange processes

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