Effect of desilication on the catalytic activity of Fe-FER for direct, selective, partial oxidation of methane

Guangyu Zhao,Penghui Yan, Kerryn Procter,Adesoji Adesina,Yonggang Jin,Eric Kennedy,Michael Stockenhuber

Journal of Catalysis（2023）

引用 3|浏览5

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摘要

•NaOH treatment enhances CH3O· groups migration from iron to silicon sites.•Diffusion and desorption of products on Fe-FER are promoted following alkaline treatment.•Stability of active oxygen species on Fe-FER can be controlled by NaOH treatment.

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关键词

Desilication,Ferrierite zeolite,Active oxygen species,Terminal silanol groups,Brønsted-acid sites,Mesopore

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