Site‐selective Multi‐Emitter Gold‐Silver Metallopolymers: A Novel Class of Self‐assembled Materials

Inés Soldevilla, Montserrat Santamaría‐Paganini,M. Elena Olmos,Miguel Monge,José M. López‐de‐Luzuriaga,María Rodríguez‐Castillo

Applied Organometallic Chemistry（2022）

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摘要

New luminescent heterometallopolymers [(Au-C6F5)(m)(AgOSO2CF3)(n) (PVP)] with different Au:Ag molar ratios were synthesized. The luminescent emissions of these polymers are strongly dependent on the temperature, excitation wavelengths, and the Au(I):Ag(I) molar ratio. The incorporation of a precise amount of Ag(I) atoms in the backbone of [(Au-C6F5)(m)(PVP)] metallopolymer allows a controlled tuning of the emission energy in the green-blue range.

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关键词

computational studies,gold(I),metallopolymers,silver(I),site-selective emitters

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