NH₂-MIL-125(Ti) with transient metal centers via novel electron transfer routes for enhancing photocatalytic NO removal and H₂ evolution

Houfan Li,Xingyan Liu,Huan Feng, Jia Zhao,Peng Lu,Min Fu,Weiwei Guo,Yi Zhao,Youzhou He

Catalysis Science & Technology（2021）

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摘要

The transient YbII/III center coordinated with –NH2 of NH2-MIL-125(Ti) to form a ligand metal charge transfer (LLCMT) pathway, which promoted the rapid transfer of electrons, thereby enhancing photocatalytic NO removal and hydrogen production.

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NH2-MIL-125(Ti) with transient metal centers via novel electron transfer routes for enhancing photocatalytic NO removal and H2 evolution

NH₂-MIL-125(Ti) with transient metal centers via novel electron transfer routes for enhancing photocatalytic NO removal and H₂ evolution