Laser-Induced Breakdown In Liquid Water: Influence Of Repeated Laser Pulses On Plasma Formation And Emission

We have experimentally investigated the influence of repeated laser pulses on laser-induced breakdown (LIB) in water following a focused 1064 nm laser pulse, for repetition rates between 0.5 and 20 Hz and up to 100 pulses. LIB plasma image data are collected as a function of repetition rate and laser pulse number, using an intensified CCD camera with sub-nanosecond camera-laser timing. Each pulse induces multiple breakdowns, shockwaves, and macroscopic cavitation bubbles. These effects disappear by the time the next pulse arrives. Even so, we find that the water target retains effects from previous pulses that persist up to roughly a second and that modify subsequent LIB properties including plasma location, spatial extension, and total emission intensity. We quantify the effects by tracking the first moment of the plasma emission intensity, which we call the "center of intensity" (CoI). Three distinct reproducible repetition-rate-dependent phases are identified with repeated pulses. In particular, (1) with initial pulses, emission intensity decreases and the CoI broadens and propagates downstream from the laser focus reaching a maximum axial distance away from the focal point, (2) with additional pulses, the CoI narrows and travels back upstream toward the laser, and (3) with continued pulses, the plasma gains back a portion of the lost intensity and the CoI reaches a steady state position, not at the focal point. Two possible causal effects are highlighted; particle inclusion concentration changes and microbubbles in the laser path.