Pd-catalyzed decarbonylation of furfural: Elucidation of support effect on Pd size and catalytic activity using in-situ XAFS

Tamao Ishida,Tetsuo Honma,Kengo Nakada,Haruno Murayama,Tetsuya Mamba,Kurumi Kume, Yusuke Izawa,Masaru Utsunomiya,Makoto Tokunaga

Journal of Catalysis（2019）

引用 31|浏览10

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摘要

•ZrO2 stabilizes Pd clusters consisting of less than 10 atoms during decarbonylation.•Single Pd atoms are inactive but Pd clusters are active species for decarbonylation.•In-situ XAFS revealed Pd13 clusters are formed on CeO2 and active in the reaction.

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关键词

In-situ XAFS,Furfural,Decarbonylation,Palladium,Heterogeneous catalyst

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