Catalytic oxidation of ethyl acetate over Ru–Cu bimetallic catalysts: Further insights into reaction mechanism via in situ FTIR and DFT studies

Xiaolong Liu,Qingzhen Han,Wenbo Shi,Cheng Zhang,Erwei Li,Tingyu Zhu

Journal of Catalysis（2019）

引用 56|浏览9

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摘要

Ruthenium-based bimetallic catalysts 1Ru–5M/TiO2 (M = Co, Ce, Fe, Mn, Cu, Ni) were prepared and evaluated in ethyl acetate oxidation. 1Ru–5Cu/TiO2 contributed the best catalytic performance. Systematic in situ FTIR and DFT studies were conducted, and a reaction mechanism for ethyl acetate oxidation over Ru–Cu bimetallic catalyst was proposed.

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关键词

Oxygenated volatile organic compounds,Ethyl acetate,Catalytic oxidation,Ruthenium,Bimetallic catalysts

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