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Inorganic
Bioinorganic
Metalloenzymes constitute a paradigmatic example of ideal catalysts. Fine tuning of the first and second coordination spheres in combination with the use of preferred readily available first row metal ions permit them to carry out a wide range of synthetic transformations. Especially relevant are the processes in which dioxygen is implicated, i) used as H+/e- acceptor to oxidize a wide range of organic substrates with an exquisite selectivity, and ii) found as final product in the photosynthetic water oxidation. In this research program, we will take inspiration of the complex enzymatic machinery to develop low-weight metal complexes that can mimic some crucial aspects of these processes. Detailed study of physical and chemical properties of relevant metal/dioxygen derived intermediate species will led to rational design of new sustainable, efficient and selective catalytic systems with useful energetic and synthetic applications beyond the enzymatic activity.
Inorganic
Bioinorganic
Metalloenzymes constitute a paradigmatic example of ideal catalysts. Fine tuning of the first and second coordination spheres in combination with the use of preferred readily available first row metal ions permit them to carry out a wide range of synthetic transformations. Especially relevant are the processes in which dioxygen is implicated, i) used as H+/e- acceptor to oxidize a wide range of organic substrates with an exquisite selectivity, and ii) found as final product in the photosynthetic water oxidation. In this research program, we will take inspiration of the complex enzymatic machinery to develop low-weight metal complexes that can mimic some crucial aspects of these processes. Detailed study of physical and chemical properties of relevant metal/dioxygen derived intermediate species will led to rational design of new sustainable, efficient and selective catalytic systems with useful energetic and synthetic applications beyond the enzymatic activity.
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Ankita Puri, Allison Mcaninch, Sheng Shu,Khashayar Rajabimoghadam,Maxime A. Siegler,Marcel Swart,Isaac Garcia-Bosch
INORGANICA CHIMICA ACTA (2024): 121844-121844
Tong Wu, Ankita Puri, Yi Lin Qiu, Daniel Ye, Rajdeep Sarma, Yiwen Wang,Tomasz Kowalewski,Maxime A Siegler,Marcel Swart,Isaac Garcia-Bosch
Inorganic chemistry (2024)
Shuming Zhang, Sunipa Goswami,Karl H. G. Schulz, Karan Gill, Xinyi Yin, Jimin Hwang, Jasmine Wiese, Isabel Jaffer,Roberto R. Gil,Isaac Garcia-Bosch
JOURNAL OF ORGANIC CHEMISTRYno. 4 (2024): 2622-2636
Tong Wu, Ankita Puri, Yi Lin Qiu, Daniel Ye, Rajdeep Sarma, Yiwen Wang,Tomasz Kowalewski,Maxime A. Siegler,Marcel Swart,Isaac Garcia-Bosch
Inorganic Chemistry (2024)
Journal of the American Chemical Societyno. 37 (2022): 16905-16915
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Handbook of CH‐Functionalizationpp.1-31, (2022)
Comprehensive Coordination Chemistry IIIpp.436-473, (2021)
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